Research on the Temporal and Spatial Characteristics of Air Pollutants in Sichuan Basin

Sichuan Basin is one of the most densely populated areas in China and the world. Human activities have great impact on the air quality. In order to understand the characteristics of overall air pollutants in Sichuan Basin in recent years, we analyzed the concentrations of six air pollutants monitored in 22 cities during the period from January 2015 to December 2020. During the study period, the annual average concentrations of CO, NO2, SO2, PM2.5 and PM10 all showed a clear downward trend, while the ozone concentration was slowly increasing. The spatial patterns of CO and SO2 were similar. High-concentration areas were mainly located in the western plateau of Sichuan Basin, while the concentrations of NO2 and particulate matter were more prominent in the urban agglomerations inside the basin. During the study period, changes of the monthly average concentrations for pollutants (except for O3) conformed to the U-shaped pattern, with the highest in winter and the lowest in summer. In the southern cities of the basin, secondary sources had a higher contribution to the generation of fine particulate matter, while in large cities inside the basin, such as Chengdu and Chongqing, air pollution had a strong correlation with automobile exhaust emissions. The heavy pollution incidents observed in the winter of 2017 were mainly caused by the surrounding plateau terrain with typical stagnant weather conditions. This finding was also supported by the backward trajectory analysis, which showed that the air masses arrived in Chengdu were mainly from the western plateau area of the basin. The results of this study will provide a basis for the government to take measures to improve the air quality in Sichuan Basin.