石墨烯
阳极
材料科学
单层
石墨
锂(药物)
堆积
纳米技术
氧化石墨烯纸
制作
异质结
电极
光电子学
化学工程
复合材料
化学
有机化学
物理化学
医学
替代医学
病理
内分泌学
工程类
作者
Xiaoliang Yu,Jie Tang,Kazuya Terabe,Taizô Sasaki,Runsheng Gao,Yoshikazu Ito,Kensuke Nakura,Kazuko Asano,Masuko Suzuki
标识
DOI:10.1016/j.matchemphys.2019.121987
摘要
Graphene materials have attracted significant research interest as anodes in lithium-ion batteries (LIBs). However, their low volumetric capacity and high working voltage limit the energy density and thus hinder their practical applications. In this research, monolayer graphene and MoS2 were prepared by controlled CVD growth processes. Graphene/MoS2 alternately stacked structure (GMASS) was subsequently fabricated by alternately stacking graphene and MoS2 monolayers layer by layer. When evaluated as an anode for LIB, GMASS demonstrates an obviously reduced working voltage compared to monolayer graphene electrodes (1.31 V vs. 1.46 V). And its volumetric capacity is much higher than that of an average graphite anode (1260 mAh cm−3 vs. 461 mAh cm−3). This fundamental research could promote the development of graphene/MoS2 heterostructures for high-energy LIBs.
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