材料科学
荧光
光致发光
显色指数
发光
发光二极管
固态
二极管
光电子学
白光
碳纤维
量子点
纳米技术
复合数
化学工程
复合材料
光学
化学
工程类
物理化学
物理
作者
Yuan Zhan,Bin Shang,Min Chen,Limin Wu
出处
期刊:Small
[Wiley]
日期:2019-05-02
卷期号:15 (24)
被引量:90
标识
DOI:10.1002/smll.201901161
摘要
Carbon dots (CDots)-based solid-state luminescent materials have important applications in light-emitting devices owing to their outstanding optical properties. However, it still remains a challenge to develop multiple-color-emissive solid-state CDots, due to the serious self-quenching of the CDots in the aggregation or solid state. Herein, a one-step synthesis of multiple-color-emissive solid-state silica-coated CDots (silica/CDots) composites by controlling CDots loading fraction and composite morphology to realize the adjustment of emitting color is reported. The emission of resultant silica/CDots composites shifts from blue to orange with the photoluminescence quantum yields of 57.9%, 34.3%, and 32.7% for blue, yellow, and orange emitting, respectively. Furthermore, the yellow emitting silica/CDots composites exhibit an excellent fluorescence thermal stability, and further have been applied to fabricate white-light-emitting devices with a high color rendering index of above 80.
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