特大城市
排放清单
环境科学
中国
污染物
人口
环境工程
环境保护
气象学
地理
空气质量指数
社会学
人口学
经济
考古
有机化学
化学
经济
作者
Shefang Wang,Shasha Yin,Xuan Lü,Binglin Zhang,Yali Liu
标识
DOI:10.1016/j.atmosres.2022.106546
摘要
Semi-volatile organic compounds (SVOCs) and intermediate volatile organic compounds (IVOCs) are key precursors for the formation of SOA, which is an important component of PM2.5, a representative pollutant of complex atmospheric pollution. It is important to understand the emissions of SVOCs and IVOCs. Based on the collected anthropogenic activity data and ratio of SVOCs and IVOCs to primary organic aerosols (POA), in this study, a newly 2017-based high-resolution S/IVOCs emission inventory in Central China represented by Henan Province was developed. The total emissions of SVOCs and IVOCs were 101.3 kt and 447.9 kt, respectively. SVOCs emission was mainly originated from residential combustion and industrial process, with the contribution of 44.4% and 20.8%, respectively. Industrial process and on-road mobile were the main contributors to IVOCs emission, accounting for 56.1% and 14.5% of total emission, respectively. This study further analyzes and compares S/IVOCs emissions of different cities based on the urban population. S/IVOCs emissions in 10 megacities, 5 large cities, and 3 small cities account for 74.9%, 16.4%, and 8.7% of total emissions, respectively. High SVOCs emissions were mainly distributed in eastern regions such as Shangqiu and Zhoukou which are agricultural cities, and that was in cities with developed industries and transportation, such as Zhengzhou and Jiaozuo, as for IVOCs. The uncertainties of SVOCs and IVOCs emissions established in this study are −60.7% - 62.2% and − 122.1% - 119.1%, respectively. Industrial process and on-road mobile are the emission sources with higher uncertainty of SVOCs and IVOCs emissions, respectively. It hopes to better understand the emission characteristics of S/IVOCs and provide more detailed basic data for air quality modelling simulation and various emission control policies.
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