升级
解耦(概率)
二氧化碳电化学还原
可再生能源
电化学
催化作用
纳米技术
材料科学
工艺工程
生化工程
环境科学
计算机科学
工程类
化学
电极
控制工程
物理化学
电气工程
操作系统
生物化学
一氧化碳
作者
Zhitong Wang,Yansong Zhou,Peng Qiu,Bao Yu Xia,Wensheng Fang,Jian Jin,Lei Huang,Peilin Deng,Ya Qiong Su,R. Crespo,Xinlong Tian,Bao Yu Xia,Wei Guo,Di Tommaso Devis,Yuanjie Pang,Shi‐Jin Ding,Bao Yu Xia
标识
DOI:10.1002/adma.202303052
摘要
Abstract Electrochemical carbon dioxide reduction reaction (CO 2 RR) driven by renewable energy shows great promise in mitigating and potentially reversing the devastating effects of anthropogenic climate change and environmental degradation. The simultaneous synthesis of energy‐dense chemicals can meet global energy demand while decoupling emissions from economic growth. However, the development of CO 2 RR technology faces challenges in catalyst discovery and device optimization that hinder their industrial implementation. In this contribution, a comprehensive overview of the current state of CO 2 RR research is provided, starting with the background and motivation for this technology, followed by the fundamentals and evaluated metrics. Then the underlying design principles of electrocatalysts are discussed, emphasizing their structure–performance correlations and advanced electrochemical assembly cells that can increase CO 2 RR selectivity and throughput. Finally, the review looks to the future and identifies opportunities for innovation in mechanism discovery, material screening strategies, and device assemblies to move toward a carbon‐neutral society.
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