等离子体子
表面等离子共振
偶极子
局域表面等离子体子
共振(粒子物理)
极化(电化学)
垂直的
分子物理学
波长
光学
纳米颗粒
半径
辐射传输
材料科学
物理
表面等离子体子
原子物理学
化学
纳米技术
几何学
量子力学
计算机科学
物理化学
计算机安全
数学
作者
Shengli Zou,Nathalie Janel,George C. Schatz
摘要
Using electrodynamics calculations, we have discovered one dimensional array structures built from spherical silver nanoparticles that produce remarkably narrow ( approximately meV or less) plasmon resonance spectra upon irradiation with light that is polarized perpendicular to the array axis. The narrow lines require a minimum particle radius of about 30 nm to achieve. Variations of the plasmon resonance wavelength, extinction efficiency and width with particle size, array structure, interparticle distance and polarization direction are examined, and conditions which lead to the smallest widths are demonstrated. A simple analytical expression valid for infinite lattices shows that the sharp resonance arises from cancellation between the single particle width and the imaginary part of the radiative dipolar interaction.
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