材料科学
石墨烯
拉曼光谱
基质(水族馆)
脉冲激光沉积
X射线光电子能谱
薄膜
无定形碳
无定形固体
碳纤维
分析化学(期刊)
通量
氢
碳膜
激光烧蚀
化学工程
激光器
纳米技术
复合材料
结晶学
化学
光学
地质学
工程类
物理
有机化学
海洋学
复合数
色谱法
作者
R.H. Benhagouga,S. Abdelli‐Messaci,M. Abdesselam,Virginie Blondeau‐Patissier,Riad Yahiaoui,M. Siad,Achour Rahal
标识
DOI:10.1016/j.apsusc.2017.07.125
摘要
A direct synthesis of hydrogenated graphene at a reduced temperature of 400° C using pulsed laser ablation technique is reported. Here, we have investigated the effect of the substrate temperature. Therefore, hydrogenated carbon thin films were elaborated under the same conditions of laser fluence and CH4 pressure but at different substrate temperatures ranging from room temperature to 600 °C. The Raman and X-ray photoelectron spectroscopy revealed a structural change induced by the substrate temperature increase. Indeed the elaborated thin films evolved from amorphous carbon to hydrogenated graphene as the substrate temperature increases. The elastic recoiled detection analysis and the Rutherford backscattering measurements indicated a decrease in the hydrogen content as well as a thickness reduction along with the substrate temperature increase. We have concluded that the structural change can be ascribed to the increase in the species mobility during the growth.
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