可再生能源
人类健康
持续性
氮气
化学
生化工程
环境科学
环境经济学
业务
纳米技术
材料科学
工程类
有机化学
生物
经济
医学
生态学
电气工程
环境卫生
作者
Peisen Liao,Jiawei Kang,Rong Xiang,Shihan Wang,Guangqin Li
标识
DOI:10.1002/anie.202311752
摘要
Abstract Inorganic nitrogen oxide (NO x ) species, such as NO, NO 2 , NO 3 − , NO 2 − generated from the decomposition of organic matters, volcanic eruptions and lightning activated nitrogen, play important roles in the nitrogen cycle system and exploring the origin of life. Meanwhile, excessive emission of NO x gases and residues from industry and transportation causes troubling problems to the environment and human health. How to efficiently handle these wastes is a global problem. In response to the growing demand for sustainability, scientists are actively pursuing sustainable electrochemical technologies powered by renewable energy sources and efficient utilization of hydrogen energy to convert NO x species into high‐value organonitrogen chemicals. In this minireview, recent advances of electrocatalytic systems for NO x species valorization in organonitrogen synthesis are classified and described, such as amino acids, amide, urea, oximes, nitrile etc., that have been widely applied in medicine, life science and agriculture. Additionally, the current challenges including multiple side reactions and complicated paths, viable solutions along with future directions ahead in this field are also proposed. The coupling electrocatalytic systems provide a green mode for fixing nitrogen cycle bacteria and bring enlightenment to human sustainable development.
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