微等离子体
纳秒
介质阻挡放电
大气压力
旋转温度
等离子体
分析化学(期刊)
非热等离子体
材料科学
体积流量
巴(单位)
喷射(流体)
化学
原子物理学
激光器
电介质
光电子学
光学
机械
物理
有机化学
色谱法
量子力学
地质学
海洋学
分子
气象学
作者
A. Elkholy,Sander Nijdam,Eddie van Veldhuizen,Nico Dam,J.A. van Oijen,Ute Ebert,L.P.H. de Goey
标识
DOI:10.1088/1361-6595/aabf49
摘要
We present a novel microplasma flow reactor using a dielectric barrier discharge (DBD) driven by repetitive nanosecond high-voltage pulses. Our DBD-based geometry can generate a non-thermal plasma discharge at atmospheric pressure and below in a regular pattern of micro-channels. This reactor can work continuously up to about 100 min in air, depending on the pulse repetition rate and operating pressure. We here present the geometry and main characteristics of the reactor. Pulse energies of 1.46 and 1.3 μJ per channel at atmospheric pressure and 50 mbar, respectively, have been determined by time-resolved measurements of current and voltage. Time-resolved optical emission spectroscopy measurements have been performed to calculate the relative species concentrations and temperatures (vibrational and rotational) of the discharge. The effects of the operating pressure and flow velocity on the discharge intensity have been investigated. In addition, the effective reduced electric field strength has been obtained from the intensity ratio of vibronic emission bands of molecular nitrogen at different operating pressures and different locations. The derived increases gradually from about 550 to 4600 Td when decreasing the pressure from 1 bar to 100 mbar. Below 100 mbar, further pressure reduction results in a significant increase in up to about 10000 Td at 50 mbar.
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