发电
材料科学
功率密度
电
致潮剂
塞贝克系数
工程物理
功率(物理)
表征(材料科学)
航程(航空)
气象学
环境科学
热力学
纳米技术
电气工程
物理
热导率
复合材料
工程类
化学
有机化学
作者
Mingchen Yang,Hao Yin,Xiaoliang Wang,Hua Chen,Jiangtao Yu,Weizheng Li,Rui Li,Feng Yan
标识
DOI:10.1002/adma.202312249
摘要
Abstract Ionic thermocells convert heat into electricity and are promising power sources for electronic devices. However, discontinuous and small electricity output limits practical use under varying environmental conditions. Here, we design a thermogalvanic ionogel with a high Seebeck coefficient (32.4 mV K −1 ). We also develop thermocells that combine thermogalvanic ionogel‐based thermocells, which realize all‐weather power generation via passive radiative cooling. These thermocells generate electricity continuously under varying weather conditions and over a wide temperature range (−40 to 90°C), with a normalized power density of 25.84 mW m −2 K −2 . Advanced characterization shows the chaotropic effect enhances the Seebeck coefficient, while the self‐supplying temperature difference given the radiative cooling structure enables all‐weather power generation. Our results provide an effective strategy for developing practical thermocells suitable for diverse daily and seasonal variations. This article is protected by copyright. All rights reserved
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