The cover artwork features an illustration of binuclear metal–organic complexes functioning like miniature robots, precisely controlling the distances between metal atoms on a macroscopic scale. In their Research Article (e202500474), Kuibo Yin, Litao Sun, Bowen Jiang, and co-workers present a strategy for accurately tuning the single-atomic interdistance from 9.3 Å to 7.0 Å and then to 6.2 Å in correlated Ru-based single-atom catalysts. This innovation unlocks a three-electron oxidation pathway for uric acid sensing.