材料科学
光电探测器
光电子学
响应度
量子效率
表面等离子共振
等离子体子
纳米颗粒
紫外线
电场
表面等离子体子
纳米技术
量子力学
物理
作者
Zhiyuan Zhang,Yanan Hu,Zhao Fu,Zihao Li,Jiadong Chen,Meng Yuan,Shaoxiong Wu,Rongdun Hong,Dingqu Lin,Xiaping Chen,Jiafa Cai,Zhengyun Wu,Yuning Zhang,Deyi Fu,Zhanwei Shen,Zhijie Wang,Feng Zhang,Rong Zhang
出处
期刊:Small
[Wiley]
日期:2025-07-04
卷期号:22 (12): e2502011-e2502011
被引量:5
标识
DOI:10.1002/smll.202502011
摘要
4H-SiC-based ultraviolet (UV) photodetectors (PDs) are urgently required for applications in flame detection and secure communication. However, these devices are hindered by their low quantum efficiency properties and sluggish response speed. Here, a substantial enhancement in UV detection is implemented by integrating periodic triangular Al/Al2O3 Core-Shell Nanoparticles (NPs) Arrays into 4H-SiC metal-semiconductor-metal (MSM) PDs. The detector exhibits an extremely low dark current (5.0 × 10-14 A) and a peak responsivity of 2.14 A W-1, corresponding to an external quantum efficiency of 984%. A high detectivity of 1.22 × 1014 Jones is achieved under illumination of 270 nm wavelength light at 30 V, while an ultra-high response speed is obtained with a rise time of 0.74 ns and a fall time of 1.47 ns. The improvement is attributed to the coupling between the lightning rod effect at the tips of the triangular NPs within the electrostatic field and localized surface plasmon resonance (LSPR), as well as the LSPR coupling effect between NPs, which enhances the electric field of the devices and triggers a localized avalanche effect. These results highlight the wide application and potential of NPs-enhanced 4H-SiC-based UV PDs in high-speed and high-precision detection.
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