罗丹明B
降级(电信)
双金属片
金属有机骨架
X射线光电子能谱
傅里叶变换红外光谱
催化作用
扫描电子显微镜
化学
环己烷
锰
化学工程
核化学
材料科学
光催化
吸附
有机化学
计算机科学
工程类
电信
复合材料
作者
Ya Li,Chong-Chen Wang,Fu-Xue Wang,Xingyuan Liu,Peng Wang,Fei Wang,Ming-Yi Sun,Baoyi Yu
出处
期刊:Dalton Transactions
[The Royal Society of Chemistry]
日期:2024-01-01
卷期号:53 (11): 5266-5273
摘要
In this work, a three-dimensional bimetallic metal-organic framework (BMOF), BUC-101 (Co/Mn-H6chhc, H6chhc = cis-1,2,3,4,5,6-cyclohexane-hexacarboxylic acid, BUC = Beijing University of Civil Engineering and Architecture) was synthesized by a one-pot solvothermal method and characterized in detail by single crystal X-ray diffraction (SCXRD), Fourier transform infrared spectroscopy (FTIR), X-ray photoelectron spectroscopy (XPS) and scanning electron microscopy (SEM) element mapping analysis. BUC-101 showed excellent catalytic peroxymonosulfate (PMS) activation performance to degrade rhodamine B (RhB) without energy input. In addition, BUC-101 can maintain good stability and recyclability during the PMS activation processes, in which 99.9% RhB degradation efficiencies could be accomplished in 5 operational runs. The possible PMS activation and RhB degradation mechanisms of the BUC-101/PMS system were proposed and affirmed.
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