Supercritical CO 2 ‐Guided Passivation Strategies for Oxygen Vacancy Modulation in LaMnO 3

The development of 2D magnetic materials and the modulation of intrinsic magnetism are essential for the exploration of new materials in the field of information storage. Despite its strong ferromagnetic properties, LaMnO₃ is hindered by a high number of oxygen defects, which result in a relatively short lifetime when employed in electronic memory devices. Here the successful transformation of bulk LaMnO₃ into a 2D structure using supercritical carbon dioxide.is reported. This technique enables the successful modulation of the magnetic properties of the material. Interestingly, it is found that the oxygen defect is repaired, which is in sharp contrast to conventional perovskites. These promising results demonstrate the potential of using the magnetic properties of LaMnO₃, which is of great importance in the context of expanding its application in electronic devices.