High-performance antibacterial tight ultrafiltration membrane constructed by co-deposition of dopamine and tobramycin for sustainable high-salinity textile wastewater management

超滤(肾) 废水 化学 化学工程 纳滤 反渗透 环境科学 环境工程 色谱法 工程类 材料科学 生物化学
作者
Wenyuan Ye,Yu Fan,Zijian Yu,Na Kong,Xiaoyan Lin,Riri Liu,Jiale Du,Xuan Huang,Ailiang Gu,Sotto Arcadio,Wenyi Zhang,Xuewei Li,Shuaifei Zhao,Ming Xie,Liang Qinghua,Jiuyang Lin
出处
期刊:Desalination [Elsevier BV]
卷期号:579: 117482-117482 被引量:19
标识
DOI:10.1016/j.desal.2024.117482
摘要

High-salinity textile wastewater is a pressing environmental concern, urgently requiring the appropriate treatment. Sustainable management of high-salinity textile wastewater via fractionation of the existing dyes and inorganic salts (NaCl) using selective separation membranes is a key approach to address this detrimental concern. Herein, tight composite ultrafiltration membranes with impressive antibacterial function were constructed using one-step co-deposition of dopamine and tobramycin on the porous substrate to fractionate the dyes and NaCl. Triggered by ammonia persulfate, the polydopamine/tobramycin coating layer imparts the fabricated composite ultrafiltration membranes with tight surface structure and narrow pore size distribution, enabling effective dyes/salts fractionation. Specifically, the tight composite ultrafiltration membrane with a molecular weight cutoff of 3692 Da experienced a > 98.0 % rejection against various reactive dyes (molecular weight: <1000 Da) with nearly complete salt transmission (<0.8 % NaCl rejection), demonstrating an effective fractionation of dyes and salts. Additionally, the incorporated tobramycin as a broad-spectrum antibiotic endowed the tight composite ultrafiltration membrane with a sufficient inhibition efficiency (i.e., 100 %) against E. coli bacteria in a short-time contact (i.e., 3 min). Thereby, the tight composite ultrafiltration membrane constructed by fast co-deposition of dopamine and tobramycin established an unparalleled platform technology for sustainable resource recovery (dyes or salts) from high-salinity textile wastewater.
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