材料科学
重复性
电容感应
氨
微波食品加热
电容
线性
聚吡咯
灵敏度(控制系统)
分析化学(期刊)
电极
化学
电子工程
电气工程
复合材料
色谱法
聚合物
物理
有机化学
量子力学
物理化学
聚合
工程类
作者
Mengxin Xu,Pan Tang,Yan-Xiong Wang,Jun-Ge Liang,Yanfeng Jiang,Pingping Yu,Tian Qiang
标识
DOI:10.1016/j.snb.2023.135248
摘要
This paper proposes a microwave transduction-based gas sensor based on polypyrrole/molybdenum oxide composite (PPy/MoO3) hybrid material. Optimization of sensing material, measurement platform and fabrication techniques are carried out to achieve excellent ammonia gas real-time detection. Capacitance parameters analysis for the gas sensing response of capacitive sensor is proceeded based on PPy, MoO3, and PPy/MoO3 hybrids at room temperature. The results show that the PPy/MoO3 hybrid material exhibits a sensitivity-enhanced response to ammonia. The PPy/MoO3 capacitive sensor has good linearity (R2=0.987), fast response, and good repeatability within 5-100 ppm ammonia concentration. Frequency parameters analysis for the gas sensing response of microwave resonator sensor is proceeded based on PPy/MoO3 hybrids in the range of 10 ppm to 100 ppm ammonia concentration at room temperature. The proposed microwave sensor has good linearity (R2=0.991), good repeatability with 8 MHz standard deviation, high stability with gas response variation less than 2%, and anti-humidity capacity. Among 100 ppm concentration of isopropanol, acetone, ethanol, methanol and ammonia, ammonia exhibits 97.5 MHz frequency shift, which proves high sensitivity and good step toward selectivity. Therefore, this work could be regarded as a promising candidate in ammonia sensing application based on microwave solution.
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