Flexible OLED Performance Enhancement: The Impact of Ag NWs: Ag NPs Electrode-Integrated MoOX QDs Hole-Injection Layer

材料科学 有机发光二极管 图层(电子) 电极 光电子学 纳米技术 化学 物理化学
作者
Zhijun Wu,Ziying Niu,Yongqiang Wang,Zijie Xu,Ke Liu,Wenjun Wang,Shuhong Li
出处
期刊:ACS Applied Materials & Interfaces [American Chemical Society]
标识
DOI:10.1021/acsami.4c20334
摘要

The growing interest in organic light-emitting diodes (OLEDs) has largely been attributed to significant performance enhancements achieved with molybdenum trioxide (MoO3). This study aims to achieve the integration of flexible transparent electrodes (FTEs) and hole-injection layers (HILs) through the use of a codoped system comprised of silver nanowires (Ag NWs) and silver nanoparticles (Ag NPs), as well as poly(3,4-ethylenedioxythiophene): poly(styrenesulfonate) (PEDOT: PSS) and molybdenum oxide quantum dots (QDs). The primary objective of this proposed technique is to use a MoO3 QD as part of a flexible electrode, reducing the step of HIL deposition in the traditional device preparation process, thereby simplifying the fabrication of flexible devices. MoO3 was reduced to MoOX, which offered an alternative pathway for hole injection to increase carrier mobility, thereby further enhancing flexible device performance. The luminance of the prepared flexible OLEDs remained at 90% of their original level, even after undergoing 500 bending tests. These findings indicate the fabricated FTEs, integrated into this system with HILs, exhibited excellent optoelectronic performance and high mechanical stability. Moreover, the structure of the flexible device with higher performance was optimized by reducing the HIL deposition process compared to traditional devices.
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