Discovery of charge density wave in a kagome lattice antiferromagnet

凝聚态物理 反铁磁性 电荷密度波 相图 超导电性 物理 充电顺序 格子(音乐) 电荷(物理) 相(物质) 量子力学 声学
作者
Xiaokun Teng,Lebing Chen,Feng Ye,Elliott Rosenberg,Zhaoyu Liu,Jia-Xin Yin,Yu-Xiao Jiang,Ji Seop Oh,M. Zahid Hasan,Kelly J. Neubauer,Bin Gao,Yaofeng Xie,M. Hashimoto,D. H. Lu,Chris Jozwiak,Aaron Bostwick,Eli Rotenberg,R. J. Birgeneau,Jiun‐Haw Chu,Ming Yi,Pengcheng Dai
出处
期刊:Nature [Springer Nature]
卷期号:609 (7927): 490-495 被引量:75
标识
DOI:10.1038/s41586-022-05034-z
摘要

A hallmark of strongly correlated quantum materials is the rich phase diagram resulting from competing and intertwined phases with nearly degenerate ground-state energies1,2. A well-known example is the copper oxides, in which a charge density wave (CDW) is ordered well above and strongly coupled to the magnetic order to form spin-charge-separated stripes that compete with superconductivity1,2. Recently, such rich phase diagrams have also been shown in correlated topological materials. In 2D kagome lattice metals consisting of corner-sharing triangles, the geometry of the lattice can produce flat bands with localized electrons3,4, non-trivial topology5-7, chiral magnetic order8,9, superconductivity and CDW order10-15. Although CDW has been found in weakly electron-correlated non-magnetic AV3Sb5 (A = K, Rb, Cs)10-15, it has not yet been observed in correlated magnetic-ordered kagome lattice metals4,16-21. Here we report the discovery of CDW in the antiferromagnetic (AFM) ordered phase of kagome lattice FeGe (refs. 16-19). The CDW in FeGe occurs at wavevectors identical to that of AV3Sb5 (refs. 10-15), enhances the AFM ordered moment and induces an emergent anomalous Hall effect22,23. Our findings suggest that CDW in FeGe arises from the combination of electron-correlations-driven AFM order and van Hove singularities (vHSs)-driven instability possibly associated with a chiral flux phase24-28, in stark contrast to strongly correlated copper oxides1,2 and nickelates29-31, in which the CDW precedes or accompanies the magnetic order.
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