环境科学
污染
分摊
健康风险评估
污染
地下水
干旱
环境卫生
环境化学
环境保护
水资源管理
环境工程
健康风险
生态学
化学
地质学
医学
岩土工程
政治学
法学
生物
作者
Shuai Du,Xiang Meng,Xin Wen,Jun Wu,Haijiao Yu,Min Wu
标识
DOI:10.1016/j.scitotenv.2022.156733
摘要
Heavy metal(loid)s accumulation in groundwater has posed serious ecological and health concerns worldwide. Source-specific risk apportionment is crucial to prevent and control potential heavy metal(loid)s pollution in groundwater. However, there is very limited comprehensive information on the health risk apportionment for groundwater heavy metal(loid)s in arid regions. Thus, the Zhangye Basin, a typical arid oasis region in Northwest China, was selected to investigate the contamination characteristics, possible pollution sources, and source-specific health risks of groundwater heavy metal(loid)s. The heavy metal pollution index (HPI), the Nemerow index (NI), and the contamination degree (CD) were adopted to assess the pollution level of heavy metal(loid)s; then source-specific health risk was apportioned integrating the absolute principal component scores-multiple linear regression (APCS-MLR) with health risk assessment. Noticeable accumulation of Mn, Fe, and As was observed in this region with especially Fe/As in 12.68%/2.11% of the samples revealing significant enrichment. Approximately 3.5% of the groundwater samples caused moderate or higher pollution level based on the HPI. The APCS-MLR model was more physically applicable for the current research than the positive matrix factorization (PMF) model. Industrial-agricultural activity factor (12.56%) was the major source of non-cancer (infants: 59.15%, children: 64.87%, teens: 64.06%, adults: 64.02%) and cancer risks (infants: 77.36%, children: 77.35%, teens: 77.40%, adults: 77.41%). Industrial-agricultural activities should be given priority to control health risks of heavy metal(loid)s in groundwater. These findings provide fundamental and significant information for mitigating health risks caused by heavy metal(loid)s in groundwater of typical arid oasis regions by controlling priority sources.
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