单线态氧
激进的
催化作用
降级(电信)
盐酸四环素
材料科学
活性氧
化学工程
电子转移
异质结
超氧化物
光化学
羟基自由基
氧气
污染物
水处理
纳米线
高级氧化法
多孔性
纳米技术
化学
比表面积
原位
多相催化
四环素
饮用水净化
硫酸盐
作者
Meiling Zhou,Haidong Zhao,Yaping Zhang,Yufeng He,Pengfei Song,Rongmin Wang
标识
DOI:10.1021/acsami.5c13873
摘要
), which collectively contribute over 90% to the degradation of tetracycline hydrochloride (TCs), achieving a removal rate of 98% within 5 min. This high efficiency is primarily attributed to the continuous generation of ROS as the dominant active species in pollutant degradation, with the heterojunction structure facilitating electron transfer and PMS activation to sustain ROS production throughout the process. Additionally, the unique wood ear-like morphology, characterized by its high aspect ratio and hierarchical porous structure, increases the surface area and exposure of active sites, facilitating mass transfer and accelerating interfacial electron interactions, thereby enhancing catalytic performance. This system also demonstrates excellent reusability, maintaining around 83% efficiency after eight cycles, and displays low biotoxicity with potential for agricultural applications. This work provides valuable insights into designing advanced catalysts for effective environmental remediation.
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