化学
纳米技术
分解水
贵金属
过渡金属
电催化剂
氮化物
碳化物
电化学
有机化学
催化作用
材料科学
物理化学
光催化
电极
图层(电子)
作者
Zonish Zeb,Yichao Huang,Lulu Chen,Wenbo Zhou,Meihong Liao,Yangyang Jiang,Haitao Li,Limin Wang,Lin Wang,Hang Wang,Tong Wei,Dejin Zang,Zhuangjun Fan,Yongge Wei
标识
DOI:10.1016/j.ccr.2023.215058
摘要
Electrocatalytic water splitting via hydrogen evolution reaction (HER) from renewable energy sources is an attractive alternative to produce hydrogen, but it still encounters the limitations of large-scale applicability of Pt-based electrocatalysts. Therefore, abundant efforts have been devoted to design and fabricate highly efficient and stable noble-metal-free electrocatalysts to replace the expensive Pt-based electrocatalysts. Recently, polyoxometalates (POMs) and their derivatives have been proven to provide plentiful opportunities for designing and fabricating highly efficient and stable noble-metal-free HER electrocatalysts with controllable catalytic active sites and well-defined nanostructures. In this review, recent advances on coordination structures and HER performances of POMs-contained composites and POMs-derived transition metal carbides, chalcogenides, phosphides, nitrides and other electrocatalysts have been discussed.
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