South and Southeast Asia controls black carbon characteristics of Meili Snow Mountains in southeast Tibetan Plateau

高原(数学) 环境科学 冰川 大气科学 气候学 大气(单位) 早晨 炭黑 自然地理学 地理 地质学 气象学 化学 数学分析 数学 医学 天然橡胶 有机化学 内科学
作者
Pengfei Chen,Shichang Kang,Yuling Hu,Tao Pu,Yajun Liu,Shijin Wang,Mukesh Rai,Ke Wang,Lekhendra Tripathee,Chaoliu Li
出处
期刊:Science of The Total Environment [Elsevier BV]
卷期号:927: 172262-172262 被引量:5
标识
DOI:10.1016/j.scitotenv.2024.172262
摘要

South and Southeast Asia (SSA) emitted black carbon (BC) exerts potential effects on glacier and snow melting and regional climate change in the Tibetan Plateau. In this study, online BC measurements were conducted for 1 year at a remote village located at the terminus of the Mingyong Glacier below the Meili Snow Mountains. The Weather Research and Forecasting model coupled with Chemistry (WRF-Chem) was used to investigate the contribution and potential effect of SSA-emitted BC. In addition, variations in the light absorption characteristics of BC and brown carbon (BrC) were examined. The results indicated that the annual mean concentration of BC was 415 ± 372 ng m−3, with the highest concentration observed in April (monthly mean: 930 ± 484 ng m−3). BC exhibited a similar diurnal variation throughout the year, with two peaks observed in the morning (from 8:00 to 9:00) and in the afternoon (from 16:00 to 17:00), with even lower values at nighttime. At a short wavelength of 370 nm, the absorption coefficient (babs) reached its maximum value, and the majority of babs values were < 20 Mm−1, indicating that the atmosphere was not overloaded with BC. At the same wavelength, BrC substantially contributed to babs, with an annual mean of 25.2 % ± 12.8 %. SSA was the largest contributor of BC (annual mean: 51.1 %) in the study area, particularly in spring (65.6 %). However, its contributions reached 20.2 % in summer, indicating non-negligible emissions from activities in other regions. In the atmosphere, the SSA BC-induced radiative forcing (RF) over the study region was positive. While at the near surface, the RF exhibited a significant seasonal variation, with the larger RF values occurring in winter and spring. Overall, our findings highlight the importance of controlling BC emissions from SSA to protect the Tibetan Plateau against pollution-related glacier and snow cover melting.
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