光催化
材料科学
光降解
纳米复合材料
X射线光电子能谱
高分辨率透射电子显微镜
拉曼光谱
煅烧
化学工程
可见光谱
水溶液
透射电子显微镜
漫反射红外傅里叶变换
比表面积
纳米技术
催化作用
光电子学
化学
光学
有机化学
物理
工程类
作者
Shuaishuai Ma,Jiandong Gu,Yingxia Han,Yuan Gao,Yuqing Zong,Zhaolian Ye,Jinjuan Xue
出处
期刊:ACS omega
[American Chemical Society]
日期:2019-12-03
卷期号:4 (25): 21063-21071
被引量:45
标识
DOI:10.1021/acsomega.9b02411
摘要
Visible-lightdriven C-TiO2 nanocomposites were prepared via a simple calcination and acid etching process. The C-TiO2 nanocomposites were characterized by X-ray photoelectron spectroscopy, Raman spectroscopy, X-ray diffraction, transmission electron microscopy, and high-resolution TEM. The results showed that TiO2 nanoparticles were combined with a porous carbon layer through surface C-O groups, which facilitates the strong interface interaction. The interface combination of nano-TiO2 and carbon material increases the specific surface area of nano-TiO2, widens the range of light response, and improves the efficiency of light-induced electron migration. The visible-light photocatalytic activity of the prepared photocatalyst was evaluated by the decomposition of tetracycline aqueous solution. Compared with that of pure TiO2, the photocatalytic activity of C-TiO2 nanocomposites was significantly improved. Furthermore, a possible photocatalytic mechanism was also tentatively proposed. This work can promote the development of active photocatalysts under solar light for the photodegradation of environmental pollutants.
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