极化子
光电子学
钙钛矿(结构)
卤化物
材料科学
激子
物理
化学
凝聚态物理
无机化学
结晶学
作者
Tingting Wang,Zhihao Zang,Yuchen Gao,Chao Lyu,Pingfan Gu,Yige Yao,Kai Peng,Kenji Watanabe,Takashi Taniguchi,Xiaoze Liu,Yunan Gao,Wei Bao,Yu Ye
出处
期刊:Nano Letters
[American Chemical Society]
日期:2022-06-17
卷期号:22 (13): 5175-5181
被引量:26
标识
DOI:10.1021/acs.nanolett.2c00906
摘要
Recently, exciton-polaritons in lead halide perovskite microcavities have been extensively investigated to address striking phenomena such as polariton condensation and quantum emulation. However, a critical step in advancing these findings into practical applications, i.e., realizing electrically pumped perovskite polariton light-emitting devices, has not yet been presented. Here, we devise a new method to combine the device with a microcavity and report the first halide perovskite polariton light-emitting device. Specifically, the device is based on a CsPbBr3 capacitive structure, which can inject the electrons and holes from the same electrode, conducive to the formation of excitons and simultaneously maintaining the high quality of the microcavity. In addition, highly polarized polariton emissions have been demonstrated due to the optical birefringence in the CsPbBr3 microplate. This work paves the way for realizing practical polaritonic devices such as high-speed light-emitting devices for information communications and inversionless electrically pumped lasers based on perovskites.
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