压气站
环境科学
甲烷
气体压缩机
甲烷排放
遥感
气象学
空间变异性
大气科学
航空航天工程
工程类
地质学
物理
化学
统计
有机化学
数学
作者
Brian Nathan,Levi M. Golston,A. S. O’Brien,Kevin Ross,William A. Harrison,Lei Tao,David J. Lary,Derek Johnson,April Covington,Nigel Clark,Mark A. Zondlo
标识
DOI:10.1021/acs.est.5b00705
摘要
A model aircraft equipped with a custom laser-based, open-path methane sensor was deployed around a natural gas compressor station to quantify the methane leak rate and its variability at a compressor station in the Barnett Shale. The open-path, laser-based sensor provides fast (10 Hz) and precise (0.1 ppmv) measurements of methane in a compact package while the remote control aircraft provides nimble and safe operation around a local source. Emission rates were measured from 22 flights over a one-week period. Mean emission rates of 14 ± 8 g CH4 s(-1) (7.4 ± 4.2 g CH4 s(-1) median) from the station were observed or approximately 0.02% of the station throughput. Significant variability in emission rates (0.3-73 g CH4 s(-1) range) was observed on time scales of hours to days, and plumes showed high spatial variability in the horizontal and vertical dimensions. Given the high spatiotemporal variability of emissions, individual measurements taken over short durations and from ground-based platforms should be used with caution when examining compressor station emissions. More generally, our results demonstrate the unique advantages and challenges of platforms like small unmanned aerial vehicles for quantifying local emission sources to the atmosphere.
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