Molybdenum Disulfide-Wrapped Carbon Nanotube-Reduced Graphene Oxide (CNT/MoS2-rGO) Nanohybrids for Excellent and Fast Removal of Electromagnetic Interference Pollution

石墨烯 材料科学 碳纳米管 氧化物 纳米技术 电磁屏蔽 二硫化钼 异质结 纳米复合材料 拉曼光谱 纳米材料 复合材料 光电子学 光学 物理 冶金
作者
Jagdees Prasad,Ashwani Kumar Singh,Amar Nath Yadav,Ajit Kumar,Monika Tomar,Amit Srivastava,Pramod Kumar,Vinay Gupta,Kedar Singh
出处
期刊:ACS Applied Materials & Interfaces [American Chemical Society]
卷期号:12 (36): 40828-40837 被引量:69
标识
DOI:10.1021/acsami.0c06219
摘要

Electromagnetic interference (EMI) pollution has now become a subject of great concern with the rapid development of delicate electronic equipment in commercial, civil, and military operations. There has been a surge in pursuit of light-weight, adaptable, effective, and efficient EMI screening materials in recent years. The present article addresses a simple and sensitive approach to synthesize a core/shell carbon nanotube/MoS2 heterostructure supported on reduced graphene oxide (CNT/MoS2-rGO nanohybrid) as an efficient electromagnetic shielding material. The structural and morphological characteristics were accessed through X-ray diffraction, transmission electron microscopy, scanning electron microscopy, and Raman spectroscopy, augmenting successful formation of the CNT/MoS2-rGO nanohybrid. The shielding performance of the as-synthesized samples has been accessed in a wide frequency range of 8–12 GHz. A CNT/MoS2-rGO nanohybrid demonstrates a better EMI shielding performance in comparison to MoS2 nanosheets and MoS2-rGO nanohybrid individually. The CNT/MoS2-rGO nanohybrid having a thickness ∼1 mm shows excellent total shielding effectiveness (SET) as high as 40 dB, whereas MoS2 and MoS2-rGO hybrid lags far, with the average value of SET as 7 and 28 dB, respectively. It also demonstrates that the nanohybrid CNT/MoS2-rGO shields the EM radiation by means of absorption through several functional defects and multiple interfaces present in the heterostructure. Herein, we envision that our results provide a simple and innovative approach to synthesize the light-weight CNT/MoS2-rGO nanohybrid having flexibility and high shielding efficiency and widen its practical applications in stealth technology.
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