自愈
抗菌剂
超分子化学
丙烯酸
材料科学
适应性
高分子化学
纳米技术
高分子科学
化学
共聚物
有机化学
复合材料
聚合物
分子
管理
医学
替代医学
病理
经济
作者
Yuanzhang Jiang,Xuyi Wang,Yanting Han,Dakai Gong,Yingchun Gu,Lin Tan
出处
期刊:Polymer
[Elsevier]
日期:2024-01-01
卷期号:290: 126516-126516
标识
DOI:10.1016/j.polymer.2023.126516
摘要
Waterborne polyurethanes (WPUs) are known for their eco-friendliness and adaptability in various industries. However, the quest for multifunctional materials has created a demand for WPUs with self-healing, recyclable, and antimicrobial properties. In this study, we introduce a universal approach to doping FeCl3 and poly(acrylic acid) (PAA) into carboxyl group containing WPUs that promotes dynamic coordination bonding between Fe3+ and -COO- groups of PAA and WPUs. WPU/Fe/PAA-5.5 with 5.5 wt % PAA stands out with excellent mechanical properties, strong self-healing capabilities and an impressive >90% antimicrobial rate. Importantly, these supramolecular films proved to be highly recyclable by facile hot-pressing, which can maintain good antimicrobial properties after multiple cycles. This research will shade light on the multifunctionalization of WPU.
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