光催化
复合材料
材料科学
辐照
纳米颗粒
可见光谱
晶体结构
兴奋剂
化学工程
纳米技术
化学
结晶学
催化作用
物理
工程类
生物化学
光电子学
核物理学
作者
Yan Li,Mengna Ding,Guoxiang Yang,Lei Wang,Liulin Luo,Yingchun Miao,Yuning Huo
标识
DOI:10.1016/j.apcata.2022.118961
摘要
Acinetobacter baumannii ( A. baumannii ) was widely existed in medical wastewater and easily induced infections to threaten the human healthy. We herein reported Ag/CoO-N photocatalyst composites for effective inactivation of A. baumannii . Ag/CoO-N composites were prepared by N-doping to CoO crystal in supercritical fluid followed with photo-reduction of Ag under visible-light irradiation. N-species was incorporated in the crystal structure of CoO, on which uniform Ag nanoparticles were stably deposited. Thus, the satisfactory photocatalytic sterilization of A. baumannii irradiated by visible-light irradiation was attributed to the high capability of light trapping and the efficient separation of photo-charges. Due to photo-induced electrons as the main active species, Ag nanoparticles and CoO-N synergistically realized mineralization of cell membrane, which lead K + ions leak from cell to crack structure of bacteria, the decrease of genetic materials, and the cripple of the self-repair function in bacteria, resulting in the final cell death. • Ag/CoO-N photocatalyst was developed for inactivation of Acinetobacter baumannii . • Ag/CoO-N was achieved via solvothermal route in supercritical fluid and photo-reduction. • Ag and CoO-N synergistically realized mineralization of bacteria cell. • K + leakage, genetic material decrease and elimination of self-repair function were achieved.
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