Deep learning: an efficient method for plasmonic design of geometric nanoparticles

Abstract Plasmons of noble metal nanoparticles have played an important role in energy transfer research, biomedical sensing, drug preparation and photocatalysis in recent years. The scattering spectra of nanoparticles are dramatically affected by numerous complex parameters, such as morphology, material, and volumes, making the parameters design a necessary step before the experiment. However, the plasmonic design is limited by several difficulties, such as the high degree of freedom, expensive trial and error costs. Herein, a plasmonic design method based on dual strategy deep learning is proposed, which can provide the design proposals according to the required spectrum. To make the model closer to the real experimental situation, the boundary element method was used to build a scattering spectra dataset of geometric nanoparticles (>1200 000 samples). Driven by the above data, the artificial intelligence (AI) model learns the relationship between spectral features and design parameters. Then, the performance statistics of the model were implemented from multiple dimensions, and a high design precision of over 90% was achieved in testing cases (testing samples >120 000). Moreover, to verify the realizability of the proposed model, the scattering spectra of nanoparticles designed by AI were constructed using a dark-field microscope system. The experimental results showed that the deviation between the target and the actual spectra was very small and within the acceptable range. This proves the realizability of the AI model proposed in this paper, and sheds light on the application of AI in plasmonic design.