Characteristics of δ13CDIC in lakes on the Tibetan Plateau and its implications for the carbon cycle

溶解有机碳 高原(数学) 碳循环 水文学(农业) 碳酸盐 碳同位素 地质学 环境科学 环境化学 总有机碳 化学 海洋学 生态学 生态系统 数学分析 有机化学 生物 岩土工程 数学
作者
Yanbin Lei,Tandong Yao,Yongwei Sheng,Enlou Zhang,Weicai Wang,Junli Li
出处
期刊:Hydrological Processes [Wiley]
卷期号:26 (4): 535-543 被引量:30
标识
DOI:10.1002/hyp.8152
摘要

Abstract Dissolved inorganic carbon isotope (δ 13 C DIC ) is an important tool to reveal the carbon cycle in lake systems. However, there are only few studies focusing on the spatial variation of δ 13 C DIC of closed lakes. Here we analyze the characteristics of δ 13 C DIC of 24 sampled lakes (mainly closed lakes) across the Qiangtang Plateau (QTP) and identify the driving factors for its spatial variation. The δ 13 C DIC value of these observed lakes varies in the range of − 15·0 to 3·2‰, with an average value of − 1·2‰. The δ 13 C DIC value of closed lakes is close to the atmospheric isotopic equilibrium value, much higher than that in rivers and freshwater lakes reported before. The high δ 13 C DIC value of closed lakes is mainly attributed to the significant contribution of carbonate weathering in the catchment and the evasion of dissolved CO 2 induced by the strong evaporation of lake water. The δ 13 C DIC value of closed lakes has a logarithmic correlation with water chemistry (TDS, DIC and pCO 2 ), also suggesting that the evapo‐concentration of lake water can influence the δ 13 C DIC value. The δ 13 C DIC value shows two opposite logarithmic correlations with lake size depending on the δ 13 C DIC range. This study suggests that the δ 13 C in carbonates in lacustrine sediments can be taken as an indicator of lake volume variation in closed lakes on QTP. Copyright © 2011 John Wiley & Sons, Ltd.
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