The evolution characteristics of surface charge on the gas–solid interface under the long-time co-action of DC-temperature gradient

电场 温度梯度 材料科学 表面电荷 电荷(物理) 电荷密度 消散 凝聚态物理 电位梯度 化学物理 分析化学(期刊) 化学 热力学 物理 物理化学 量子力学 色谱法
作者
Yi Zhang,Bo Qi,Xiao Yang,Xin Wang,Zhuodong Yang,Licheng Lu,Chengrong Li
出处
期刊:Journal of Physics D [IOP Publishing]
卷期号:56 (3): 034003-034003 被引量:2
标识
DOI:10.1088/1361-6463/aca33d
摘要

Abstract The charge accumulation phenomenon at the gas–solid interface under the co-action of DC electric field and temperature gradient is of great significance, but its long-time evolution characteristics are still unclear. In this work, the accumulation and dissipation characteristics of the surface charge on the epoxy-SF 6 interface within 216 h were obtained, indicating that, (a) the normal surface electric field is increased by the temperature gradient along the gas–solid interface, which results in a prominent increase in the surface charge density; (b) there are different evolution processes of surface charge in high and low temperature regions under the co-action of DC-temperature gradient, and the increase of the charge trap density caused by the degradation of solid material is considered to be an important reason for the charge evolution; (c) the total charge dissipation ratio within 600 s decreases with the increase of charging time in DC electric field, and the surface charge dissipates mainly to the gas side of the interface; (d) the large amount of charge accumulated at the interface distorts the surface electric field at the triple junction points. The total electric field strength at the low-temperature tri-junction point increases by 35.5%, while the direction of the tangential field at the high-temperature tri-junction point reverses during the long-time co-action of the DC-temperature gradient. The results of this work may be helpful to understand the long-time charge evolution characteristics of the gas–solid interface under the DC-temperature gradient and to reveal the failure mechanism of the gas–solid interface.
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