纳米复合材料
光催化
光降解
吸附
水溶液
可重用性
材料科学
化学工程
金属有机骨架
降级(电信)
催化作用
纳米技术
化学
有机化学
计算机科学
工程类
电信
程序设计语言
软件
作者
Jiafei Wu,Xiuxuan Fang,Yingzhi Zhu,Na Ma,Wei Dai
出处
期刊:Energy & Fuels
[American Chemical Society]
日期:2020-09-14
卷期号:34 (10): 12911-12917
被引量:27
标识
DOI:10.1021/acs.energyfuels.0c02485
摘要
A good design of efficient metal-organic framework material (MOF)-based photocatalysts with high intrinsic activity for tetracycline (TC) is highly desirable, but challenging, for water purification. Herein, we have constructed a novel TiO2@UiO-66-NH2 nanocomposite through a convenient one-step solvothermal technique. The TiO2@UiO-66-NH2 nanocomposite displayed outstanding adsorption and photodegradation performances toward TC in aqueous solution under restricted space and visible light illumination. The improved catalytic ability was mainly caused by the enhanced adsorption property and the successful transfer of photogenerated electrons to the conduction band of TiO2@UiO-66-NH2. Importantly, the photocatalyst efficiency was not tremendously decreased even after the fourth round of recycling, indicating its good stability and reusability. We believe that our study could be conducive to the future design and accomplishment of MOF surface interactions with organic pollutants, expanding the application of MOFs and photocatalysts for elimination of pollutants from wastewater.
科研通智能强力驱动
Strongly Powered by AbleSci AI