Advancements and Strategies in CsPbI2Br Perovskite Solar Cells for Enhanced Efficiency and Stability

In recent years, inorganic perovskite solar cells (IPSCs), especially those based on CsPbI₂Br, have attracted considerable attention owing to their exceptional thermal stability and a well-balanced combination of light absorption and phase stability. This review provides an extensive overview of the latest progress in CsPbI₂Br PSCs, focusing on film deposition techniques, crystallization control, interface engineering, and charge transport layers (CTLs). High-efficiency CsPbI₂Br PSCs can be achieved through the optimization of these key aspects. Various strategies, such as solvent engineering, component/additive engineering, and interface optimization, have been explored to enhance the quality of CsPbI₂Br films and improve device performance. Despite significant progress, challenges remain, including the need for even higher quality films, a deeper understanding of interface energetics, and the exploration of novel CTLs. Additionally, long-term stability continues to be a critical concern. Future research should focus on refining film preparation methods, developing sophisticated interfacial layers, exploring compatible charge transport materials, and ensuring device durability through encapsulation and moisture-resistant materials.