纤维素
塞贝克系数
热电效应
材料科学
化学工程
热电发电机
电解质
超级电容器
复合材料
化学
电容
电极
热导率
热力学
物理化学
物理
工程类
作者
Yang Hu,Minzhang Chen,Chaoran Qin,Jipeng Zhang,Ang Lu
标识
DOI:10.1016/j.carbpol.2022.119650
摘要
Natural polymer-based thermoelectric materials are significant for sustainable development because they can be used to directly harvest heat into electricity while avoiding the utilization of petroleum-based resources. Herein, cellulose ionic conductors were fabricated by using cellulose as the hydrogel matrix and cellulose solvents as the electrolytes. p-type and n-type thermoelectric generators (TEG) based on cellulose ionic conductor were obtained, with Seebeck coefficient of 2.61 and -1.33 mV/K, due to the different interactions between quaternary ammonium cations and cellulose. The cellulose TEG-based supercapacitor showed a high specific capacitance and the ability of charging with thermal energy and powering electronic devices with a maximum power density of 0.42 mW/m2. Moreover, a flexible module-type TE harvester with 10 pairs of p-n legs was assembled for body heat harvesting, delivering a thermovoltage of 0.42 V for a temperature gradient of 13 K, enabling waste/biological heat conversion, temperature monitoring and temperature control.
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