Highly sensitive, reliable and flexible pressure sensor based on piezoelectric PVDF hybrid film using MXene nanosheet reinforcement

The rapid advances in intelligence terminal devices have raised expectations for highly sensitive, reliable and flexible pressure sensor. Herein, we present a highly sensitive flexible pressure sensor based on piezoelectric MXene/poly(vinylidene fluoride) (PVDF) hybrid film. Making use of MXene nanosheet reinforcement, one can efficiently promote the piezoelectric output and consequently sensitivity of PVDF. For instance, upon a small loading of 0.4 wt%, the piezoelectric coefficient d33 of MXene/PVDF hybrid film reaches the peak of 43 pC/N. Meanwhile, the incorporation of MXene nanosheet is advantageous to strengthen the mechanical performance of PVDF. With the excellent piezoelectric response and mechanical property, the MXene/PVDF hybrid film sensor demonstrates to perform superior voltage sensitivity up to 0.0480 V/N, which is double that of PVDF based sensor. Meanwhile, the novel hybrid film sensor also exhibits fast recovery time of 3.1 ms and stable operation capability under cyclic force, confirming their applicability as reliable pressure sensor.