材料科学
钙钛矿(结构)
能量转换效率
制作
光电子学
堆栈(抽象数据类型)
化学工程
涂层
光伏系统
复合材料
工程类
生物
病理
医学
程序设计语言
替代医学
计算机科学
生态学
作者
Jin Hyuck Heo,Fei Zhang,Chuanxiao Xiao,Su Jeong Heo,Jin Kyoung Park,Joseph J. Berry,Kai Zhu,Sang Hyuk Im
出处
期刊:Joule
[Elsevier]
日期:2021-02-01
卷期号:5 (2): 481-494
被引量:75
标识
DOI:10.1016/j.joule.2020.12.010
摘要
Inorganic perovskite solar cells (PSCs) are promising for achieving long-term operational stability with good device performance. Here, we report the fabrication of inorganic CsPbI2Br-based perovskite thin films with a well-defined CsPbI3−xBrx composition gradient in the surface region by a scalable, orthogonal processable spray-coating approach. The graded structure broadens absorption wavelength range and increases carrier lifetime, but it also causes electrical field redistribution within a device stack for more efficient charge separation and collection. With this approach, we obtained a power conversion efficiency of 16.81% for a 0.096-cm2 PSC. We further demonstrated a monolithically integrated perovskite submodule based on the graded CsPbI3−xBrx by spray coating with an efficiency of 13.82% (112-cm2 aperture area) and ∼9% degradation over 1,000-h continuous 1-sun light soaking.
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