Multifunctional Flexible Ionic Skin with Dual-Modal Output Based on Fibrous Structure

Flexible wearable electronic devices with multiple sensing functions that simulate human skin in all aspects have become a popular research topic. However, the current expensive and time-consuming means of integration and the complex decoupling process are hampering the further development of multifunctional sensors. Here, an ultraflexible ionic fiber membrane (IFM) prepared by a simple electrospinning technique is reported, which exhibits pressure and humidity sensing properties. With the help of different electrode structures, the IFM-based multifunctional sensor achieved pressure and humidity detection with different sensing mechanisms. Pressure sensing with high sensitivity (49.7 kPa –1 at 0–30 kPa) and wide detection range (0–220 kPa) was indicated by the capacitive signal. Humidity sensing with high linearity (1.086% per percent relative humidity (RH)) in the range 15%–90% RH was indicated by the resistance signal. In particular, the multimodal output of capacitance/resistance corresponding to pressure/humidity in this study directly addresses the problem of accurately distinguishing the two stimuli. Furthermore, we have demonstrated that the impact between pressure and humidity is negligible when measured simultaneously and independently. Because of the excellent pressure/humidity sensing performance, we have fabricated a smart bracelet and mask for pulse, skin moisture, and breathe monitoring, which indicates the promising future of multifunctional flexible sensors based on IFM in the healthcare field.