MXene‐Based Pressure Sensor with a Self‐Healing Property for Joule Heating and Friction Sliding

Abstract As a kind of flexible electronic device, flexible pressure sensor has attracted wide attention in medical monitoring and human‐machine interaction. With the continuous deepening of research, high‐sensitivity sensor is developing from single function to multi‐function. However, Current multifunctional sensors lack the ability to integrate joule heating, detect sliding friction, and self‐healing. Herein, a MXene/polyurethane (PU) flexible pressure sensor with a self‐healing property for joule heating and friction sliding is fabricated. The MXene/PU sensitive layer with special spinosum structure is prepared by a simple spraying method. After face‐to‐face assembly of the sensitive layers, the MXene/PU flexible pressure sensor is obtained and showed excellent sensitivity (150.65 kPa −1 ), fast response/recovery speed (75.5/63.9 ms), and good stability (10 000 cycles). Based on the self‐healing property of PU, the sensor also has the ability to heal after mechanical damage. In addition, the sensor realizes the joule heating function under low voltage, and has the real‐time monitoring ability of sliding objects. Combined with low cost and simple manufacturing method, the multi‐functional MXene/PU flexible sensor shows a wide range of application potential in human activity monitoring, thermal management, and slip recognition.