解吸
水溶液
溶剂
体积流量
化学
体积热力学
化学工程
工艺工程
工作(物理)
材料科学
热力学
有机化学
物理
工程类
吸附
作者
Subhajit Dutta,Sangram Roy,Xiaojun Lang,Siyuan Chen,Rohit Kumar,Chanchal Loha,Tom Verspeelt,Kevin M. Van Geem,Geraldine J. Heynderickx,Yi Ouyang
标识
DOI:10.1021/acs.iecr.4c00904
摘要
Solvent regeneration is a pivotal component in CO 2 capture technology, primarily due to its high energy consumption, which constitutes the most significant cost factor. In the present study, the application of the gas–liquid vortex reactor (GLVR) as a new process intensification (PI) technology for solvent regeneration is introduced. An experimental study of the regeneration of a 30-weight percentage (wt %) monoethanolamine (MEA) aqueous solution loaded with CO 2 is performed. The most important process conditions are studied experimentally, including gas flow rate (15 to 25 N m 3 /h), liquid flow rate (20–40 kg/h), and CO 2 loading of the MEA aqueous solution (0.28–0.49 mol of CO 2 /mol of MEA). In this operational range, the desorption efficiency peaks at 74%. As a first assessment of its use, this work adopts the CO 2 release rate per unit volume of the reactor as a key performance indicator to compare GLVR technology with other PI technologies. Our findings indicate that the CO 2 release rate in the GLVR significantly surpasses that of benchmark technology, demonstrating its potential as a more efficient alternative to solvent regeneration technology.
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