胺气处理
溶剂
环境科学
过程(计算)
发电站
工艺工程
碳纤维
哌嗪
生物量(生态学)
大气(单位)
计算机科学
生化工程
化学
有机化学
环境工程
工程类
气象学
算法
物理
复合数
电气工程
操作系统
海洋学
地质学
作者
Kevin Maik Jablonka,Charithea Charalambous,Eva Sánchez Fernández,Georg Wiechers,Juliana Garcia Moretz‐Sohn Monteiro,Peter Moser,Berend Smit,Susana García
出处
期刊:Science Advances
[American Association for the Advancement of Science]
日期:2023-01-04
卷期号:9 (1)
被引量:20
标识
DOI:10.1126/sciadv.adc9576
摘要
One of the main environmental impacts of amine-based carbon capture processes is the emission of the solvent into the atmosphere. To understand how these emissions are affected by the intermittent operation of a power plant, we performed stress tests on a plant operating with a mixture of two amines, 2-amino-2-methyl-1-propanol and piperazine (CESAR1). To forecast the emissions and model the impact of interventions, we developed a machine learning model. Our model showed that some interventions have opposite effects on the emissions of the components of the solvent. Thus, mitigation strategies required for capture plants operating on a single component solvent (e.g., monoethanolamine) need to be reconsidered if operated using a mixture of amines. Amine emissions from a solvent-based carbon capture plant are an example of a process that is too complex to be described by conventional process models. We, therefore, expect that our approach can be more generally applied.
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