铜
催化作用
氧化还原
选择性
纳米技术
合金
温室气体
材料科学
冶金
化学
方位(导航)
工艺工程
化学工程
环境科学
计算机科学
工程类
有机化学
人工智能
生物
生态学
作者
Zhiyi Sun,Yaning Hu,Danni Zhou,Mengru Sun,Shuo Wang,Wenxing Chen
出处
期刊:ACS energy letters
[American Chemical Society]
日期:2021-10-23
卷期号:6 (11): 3992-4022
被引量:59
标识
DOI:10.1021/acsenergylett.1c01965
摘要
In the face of the increasingly serious greenhouse effect and climate warming, carbon dioxide reduction (CO2RR) technology, which can produce valuable chemicals and fuels while consuming CO2, has become the focus of technology development. However, in the process of CO2 conversion into high-value products, it is still a challenge for electrocatalytic materials to achieve high efficiency and selectivity while inhibiting the byproducts of the hydrogen evolution reaction. These challenges can be solved by clarifying the factors regulating the catalytic performance of the CO2RR. With this background, we divided copper-bearing catalysts into bulk phase catalyst, copper-bearing compound catalyst, alloy catalyst, and single-atom catalyst and summarized the development status of each system in recent years. In addition, we further discussed the mechanisms affecting the performance of the CO2RR to help design catalysts with more effective selectivity. We hope this Review will inspire and encourage researchers to develop copper-bearing catalysts with better CO2RR performance.
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