电化学
催化作用
价(化学)
纳米颗粒
产量(工程)
金属
化学工程
法拉第笼
材料科学
化学
纳米技术
无机化学
电极
物理化学
冶金
有机化学
物理
量子力学
磁场
工程类
作者
Xuliang Pang,Yifei Huang,Huaiquan Zhao,Weiqiang Fan,Hongye Bai
摘要
To induce the generation of active species at the metal-carrier interface, a new synthetic strategy was successfully developed to reconstruct the Ni MOF-Au via electrochemical activation. This unique configuration not only obtained high-valence NiOOH-Au3+ species, but also stably anchored the Au nanoparticles on the surface of the catalyst. As a result, nearly 99.8% FDCA yield and 100% Faraday efficiency of FDCA were achieved at the optimal potential of 1.57 V vs. RHE. Therefore, this electrochemical reconstruction provides new insights for the development of efficient catalysts in other heterogeneous catalytic reactions.
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