催化作用
电极
阳极
可逆氢电极
析氧
克拉克电极
镍
膜电极组件
钯氢电极
化学工程
化学
材料科学
工作电极
电化学
工程类
有机化学
冶金
电解质
物理化学
作者
Ji Eun Park,Sung-Bin Park,Mi-Ju Kim,Hyun-Seop Shin,Sun Young Kang,Yong‐Hun Cho,Yung‐Eun Sung
标识
DOI:10.1021/acscatal.1c04117
摘要
The design of high-performance and durable electrodes for the oxygen evolution reaction (OER) is crucial for anion-exchange membrane water electrolyzers (AEMWE). Herein, a three-dimensional unified electrode in which nickel–iron oxyhydroxide (NiFeOOH) is directly electrodeposited on a gas diffusion layer (GDL) is developed as an AEMWE anode. Unlike conventional electrodes with a separate catalyst layer and GDL, the unified electrode comprises a single component integrating the catalyst layer with the GDL. The resulting unified electrode shows higher catalytic activity than a conventional electrode based on commercial NiFe and IrO2 and stable activity over 500 h. Investigation of the electrode parameters revealed an outstanding AEMWE performance of 3600 mA cm–2 at 1.9 V, which is the highest among many AEMWE studies. The unified AEMWE also showed durable performance at an ultrahigh current density. Therefore, unified electrode design can be considered an alternative to conventional electrodes to reduce the hydrogen production cost.
科研通智能强力驱动
Strongly Powered by AbleSci AI