Solidification of heavy metals in municipal solid waste incineration washed fly ash by asphalt mixture

粉煤灰 沥青 焚化 浸出(土壤学) 毒性特征浸出程序 废物管理 城市固体废物 底灰 焚烧炉底灰 材料科学 冶金 环境污染 环境科学 复合材料 金属 环境保护 土壤科学 工程类 土壤水分
作者
Yue Wang,Ruiping Li,Jiangang Qiao
出处
期刊:Chemosphere [Elsevier BV]
卷期号:343: 140281-140281 被引量:1
标识
DOI:10.1016/j.chemosphere.2023.140281
摘要

Using asphalt mixture to solidify heavy metals in municipal solid waste incineration fly ash can reduce pollution and realize resource utilization. In this study, the physical and chemical properties of washed fly ash were analyzed, and washed fly ash was added to asphalt mixture as filler instead of mineral powder. The study involved analyzing the mechanical attributes of asphalt mixtures containing washed fly ash, along with examining the characteristics of asphalt binder that incorporates the washed fly ash. Subsequently, assess the potential leaching hazards associated with asphalt mixture incorporating washed fly ash. The test results showed that washed fly ash was a Si-Al-Ca system material, which had small particle size, large specific surface area and many pores. It increased the contact area with asphalt, which improved encapsulation of asphalt and aggregates. The optimal dosage of washed fly ash is 2.5%. At this dosage, the mixture attains optimal high-temperature performance, while both low-temperature performance and the characteristics of washed fly ash asphalt binder align with requirements. Asphalt mixture has solidification on heavy metals, with strongest solidification for Zn, followed by Cu, Cr. A prediction model of leaching amount versus time was constructed for Pb, Ba and Ni, which have weak solidified ability. The cumulative leaching amount of the road within 15 years of service life was calculated through the model, and it was obtained that the addition of washed fly ash will not cause pollution to environment. Overall, this study showed that asphalt mixtures can be used for stabilization/solidification of washed fly ash while saving natural mineral, providing a theoretical basis for the resource application of washed fly ash in asphalt road construction.
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