Graphene oxide-based efficient and scalable solar desalination under one sun with a confined 2D water path

海水淡化 海水淡化 石墨烯 太阳能淡化 路径(计算) 工艺工程 可扩展性 氧化物 材料科学 环境科学 太阳能蒸馏器 环境工程 计算机科学 化学工程 纳米技术 工程类 化学 计算机网络 冶金 数据库 生物化学
作者
Xiuqiang Li,Weichao Xu,Mingyao Tang,Lin Zhou,Bin Zhu,Shining Zhu,Jia Zhu
出处
期刊:Proceedings of the National Academy of Sciences of the United States of America [National Academy of Sciences]
卷期号:113 (49): 13953-13958 被引量:1231
标识
DOI:10.1073/pnas.1613031113
摘要

Because it is able to produce desalinated water directly using solar energy with minimum carbon footprint, solar steam generation and desalination is considered one of the most important technologies to address the increasingly pressing global water scarcity. Despite tremendous progress in the past few years, efficient solar steam generation and desalination can only be achieved for rather limited water quantity with the assistance of concentrators and thermal insulation, not feasible for large-scale applications. The fundamental paradox is that the conventional design of direct absorber-bulk water contact ensures efficient energy transfer and water supply but also has intrinsic thermal loss through bulk water. Here, enabled by a confined 2D water path, we report an efficient (80% under one-sun illumination) and effective (four orders salinity decrement) solar desalination device. More strikingly, because of minimized heat loss, high efficiency of solar desalination is independent of the water quantity and can be maintained without thermal insulation of the container. A foldable graphene oxide film, fabricated by a scalable process, serves as efficient solar absorbers (>94%), vapor channels, and thermal insulators. With unique structure designs fabricated by scalable processes and high and stable efficiency achieved under normal solar illumination independent of water quantity without any supporting systems, our device represents a concrete step for solar desalination to emerge as a complementary portable and personalized clean water solution.
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