材料科学
金属锂
锂(药物)
阳极
制作
金属
基质(水族馆)
铁磁性
碱金属
电解质
纳米技术
电极
冶金
凝聚态物理
物理
量子力学
地质学
病理
海洋学
替代医学
内分泌学
物理化学
化学
医学
作者
Wangyan Wu,Zhenyou Song,Yiming Dai,Xueying Zheng,Guangyu Chai,Jingbi Yang,Wei Luo
标识
DOI:10.1002/aenm.202200999
摘要
Abstract Lithium metal anodes may allow the energy density limit of rechargeable lithium batteries to be pushed higher. However, simple and efficient processing technologies for thin Li metal are lacking, which has significantly limited its applications. Herein, the feasibility of engineering Li metal by compositing it with ferromagnetic particles (termed magnetic Li, abbr. M‐Li) is reported. Due to its magnetic response, straightforward processing of M‐Li on diverse substrates with customized patterns and desired thickness is realized. Moreover, when a garnet‐type solid‐state electrolyte Li 6.5 La 3 Zr 1.5 Ta 0.5 O 12 (LLZTO) is the substrate, intimate contact between M‐Li and LLZTO is obtained, with a low interfacial resistance of ≈11 Ω cm 2 . In addition to facilitating movement and wetting on various substrates, magnetic transfer of M‐Li sheets to designated locations is also enabled. The intriguing and brand‐new method for Li metal engineering via magnetic actuation may be adopted by the industrial system for the fabrication of Li metal batteries, extended to other alkali metals and promises further progress.
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