超导电性
单斜晶系
凝聚态物理
材料科学
金属
相变
环境压力
格子(音乐)
相(物质)
超导转变温度
电荷密度波
结晶学
物理
晶体结构
热力学
化学
冶金
量子力学
声学
作者
Jing Guo,Cheng Huang,Huixia Luo,Huaixin Yang,Linlin Wei,Shu Cai,Yazhou Zhou,Hengcan Zhao,Xiaodong Li,Yanchun Li,Ke Yang,Aiguo Li,Peijie Sun,Jianqi Li,Qi Wu,R. J. Cava,Liling Sun
标识
DOI:10.1103/physrevmaterials.6.l051801
摘要
Transition metal dichalcogenides host a wide variety of lattice and electronic structures, as well as corresponding exotic physical properties, especially under certain tuning conditions. Here, we report the observation of pressure-induced three superconducting transitions in ${\mathrm{TaTe}}_{2}$, a charge density wave (CDW)--bearing layered transition-metal dichalcogenide that is metallic but not superconducting at ambient pressure. We find that its CDW state can be easily suppressed upon increasing pressure up to \ensuremath{\sim}1 GPa. A superconducting state then emerges from the suppressed CDW state and persists to the pressure about 7 GPa. Unexpectedly, another superconducting state appears at \ensuremath{\sim}11 GPa within the same monoclinic (M) structure of its ambient-pressure one. Upon further compression to 21 GPa, a third superconducting state with higher ${T}_{c}$ appears from a high-pressure (HP) phase. Our experimental results suggest that the pressure-induced three superconducting transitions in ${\mathrm{TaTe}}_{2}$ are, respectively, driven by the suppression of the CDW state, the change of the \ensuremath{\beta} angle in the M phase and the transition of M-to-HP phase. These results demonstrate not only the versatile nature of this correlated electron system, but also the first experimental example that shows the pressure-induced evolution from a CDW state to three superconducting states driven by different mechanisms.
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