光催化
化学
光化学
降级(电信)
猝灭(荧光)
电子顺磁共振
诺氟沙星
化学工程
抗生素
荧光
催化作用
环丙沙星
有机化学
量子力学
生物化学
电信
物理
计算机科学
工程类
核磁共振
作者
Chen Li,Tianyi Sun,Guohui Yi,Da‐Shuai Zhang,Yan Zhang,Xiaoxue Lin,Jinrui Liu,Zaifeng Shi,Qiang Lin
出处
期刊:Molecules
[MDPI AG]
日期:2023-02-07
卷期号:28 (4): 1597-1597
被引量:2
标识
DOI:10.3390/molecules28041597
摘要
In this paper, the photocatalytic degradation efficiency of typical antibiotics (norfloxacin (NOR), sulfamethoxazole (SMX) and tetracycline hydrochloride (TCH)) by Ag/CNQDs/g-C3N4 under visible light irradiation was studied. Various strategies were applied to characterize the morphology, structure and photochemical properties of the Ag/CNQDs/g-C3N4 composites. The superior photocatalytic activity of Ag/CNQDs/g-C3N4 was attributed to the wide light response range and the enhancement of interfacial charge transfer. At the same time, the effect of the influence factors (pH, Humic acid (HA) and coexisting ions) on the antibiotics degradation were also investigated. Furthermore, the electron spin resonance (ESR) technology, free radical quenching experiments, LC/MS and DFT theoretical calculations were applied to predict and identify the active groups and intermediates during the photocatalytic degradation process. In addition, Ag/CNQDs/g-C3N4 exhibited the obvious antibacterial effect to Escherichia coli due to the addition of Ag NPs. This study develops a new way for the removal of emerging antibiotic pollution from wastewaters.
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