Development of silver oxide-loaded reduced graphene oxide nanohybrids for enhanced photocatalytic activity under visible light in aqueous solutions

光催化 光降解 材料科学 石墨烯 纳米复合材料 氧化物 罗丹明B 化学工程 可见光谱 水溶液 X射线光电子能谱 纳米材料 纳米颗粒 纳米技术 化学 催化作用 有机化学 冶金 光电子学 工程类
作者
Velu Manikandan,G. Palanisamy,Jintae Lee,Mohammed Fahad Albeshr,Abdulwahed Fahad Alrefaei,L. Arul Pragasan,Fuchun Zhang,Xinghui Liu
出处
期刊:Chemosphere [Elsevier BV]
卷期号:336: 139227-139227 被引量:3
标识
DOI:10.1016/j.chemosphere.2023.139227
摘要

We report on the synthesis of silver oxide/reduced graphene oxide nanocomposites (Ag/rGO NCs) using a hydrothermal technique. This paper presents a simple method for synthesizing Ag/rGO hybrid nanocomposites, which can be used for environmentally treating hazardous organic pollutants. The photocatalytic degradation of model artificial Rhodamine B dye and bisphenol A was assessed under visible light illumination. The crystallinity, binding energy, and surface morphologies of the synthesized samples were determined. The silver oxide loading sample resulted in a decrease in the rGO crystallite size. SEM and TEM images demonstrate strong adhesion of the Ag NPs to the rGO sheets. XPS analysis validated the binding energy and elemental composition of the Ag/rGO hybrid nanocomposites. The objective of the experiment was to enhance the photocatalytic efficiency of rGO in the visible region using Ag nanoparticles. The synthesized nanocomposites in the visible region exhibited good photodegradation percentages of approximately 97.5% and 98.6% after 120 min of irradiation for pure rGO, Ag NPs, and Ag/rGO nanohybrid, respectively. Furthermore, the Ag/rGO nanohybrid maintained their degradation ability for up to three cycles. The synthesized Ag/rGO nanohybrid demonstrated enhanced photocatalytic activity, expanding their potential for environmental remediation. Based on the investigations, Ag/rGO nanohybrid proved to be an effective photocatalyst and holds promise as an ideal material for future applications in preventing water pollution.
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