材料科学
催化作用
表征(材料科学)
选择性
Atom(片上系统)
氧还原反应
还原(数学)
生化工程
纳米技术
计算机科学
化学
物理化学
工程类
有机化学
电化学
嵌入式系统
几何学
数学
电极
作者
Yiran Ying,Xin Luo,Jinli Qiao,Haitao Huang
标识
DOI:10.1002/adfm.202007423
摘要
Abstract Double‐atom catalysts (DACs) have emerged as a novel frontier in heterogeneous catalysis because the synergistic effect between adjacent active sites can promote their catalytic activity while maintaining high atomic utilization efficiency, good selectivity, and high stability originating from the atomically dispersed nature. In this review, the recent progress in both experimental and theoretical research on DACs for various catalytic reactions is focused. Specifically, the central tasks in the design of DACs—manipulating the synergistic effect and engineering atomic and electronic structures of catalysts—are systematically reviewed, along with the prevailing experimental, characterization, and computational modeling approaches. Furthermore, the practical applications of DACs in water splitting, oxygen reduction reaction, nitrogen reduction reaction, and carbon dioxide reduction reaction are addressed. Finally, the future challenges for DACs are summarized and an outlook on the further investigations of DACs toward heterogeneous catalysis in high‐performance energy and environmental applications is provided.
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